March 2025

Journal

Assessing the coating implications of slurry formulations in NCMA and LFMP blend cathodes for lithium-ion batteries

By:
Bisht, Anuj ; Belharouak, Ilias ; Dixit, Marm B; Abouimrane, Ali ; Amin, Md Ruhul ; Sawicki, Conrad H; Steenman, Teresa E; Essehli, Rachid ; Hagh, Nader; Viswanathan, Umamaheswari
Journal Name:
Journal of Power Sources
Page Number:
236734
Volume:
640
Publication Date:
March 14, 2025
View DOI Listing:
https://doi.org/10.1016/j.jpowsour.2025.236734

Abstract

This paper investigates the implications of slurry formulations and electrode processing on the performance of lithium-ion battery (LIB) cathodes, focusing on Nickel Cobalt Manganese Aluminum (NCMA) and Lithium Ferro Manganese Phosphate (LFMP) blends. Through a comprehensive examination of electrode processing steps, from material selection to coating application, we elucidate the critical role of processing parameters in shaping electrode morphology and electrochemical behavior. Rheological studies reveal the influence of slurry composition on viscosity and flow behavior, highlighting the importance of achieving optimal rheological properties for uniform coating deposition. Electrochemical characterization, including cyclic voltammetry and rate capability tests, unveils the electrochemical behavior of NCMA, LFMP, and their blend, showcasing the synergistic effects of material blending on battery performance. Our findings underscore the intricate relationship between slurry formulation, electrode processing, and LIB performance, offering valuable insights for the design and optimization of high-performance electrode materials for next-generation batteries.