Compound-Nucleus and Doorway-State Decays of 𝛽-Delayed Neutron Emitters 51,52,53K

Abstract

We investigated decays of 51,52,53K at the ISOLDE Decay Station at CERN in order to understand the mechanism of the 𝛽-delayed neutron-emission (𝛽⁢𝑛) process. The experiment quantified neutron and 𝛾-ray emission paths for each precursor. We used this information to test the hypothesis, first formulated by Bohr in 1939, that neutrons in the 𝛽⁢𝑛 process originate from the structureless “compound nucleus.” The data are consistent with this postulate for most of the observed decay paths. The agreement, however, is surprising because the compound-nucleus stage should not be achieved in the studied 𝛽 decay due to insufficient excitation energy and level densities in the neutron emitter. In the 53K 𝛽⁢𝑛 decay, we found a preferential population of the first excited state in 52Ca that contradicted Bohr’s hypothesis. The latter was interpreted as evidence for direct neutron emission sensitive to the structure of the neutron-unbound state. We propose that the observed nonstatistical neutron emission proceeds through the coupling with nearby doorway states that have large neutron-emission probabilities. The appearance of “compound-nucleus” decay is caused by the aggregated small contributions of multiple doorway states at higher excitation energy.